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논문 기본 정보
- 자료유형
- 학술저널
- 저자정보
- 발행연도
- 2016.9
- 수록면
- 231 - 236 (6page)
- DOI
- 10.15531/ksccr.2016.7.3.231
이용수
초록· 키워드
오류제보하기
Electrocatalytic reduction can produce useful chemicals and fuels such as carbon monoxide, methane, formate, aldehydes, and alcohols using carbon dioxide, the green house gas, as a reactant through the supply of electrical energy. In this study, tin-lead (Sn-Pb) alloy electrodes are fabricated by electrodeposition on a carbon paper with different alloy composition and used as cathode for electrocatalytic reduction of carbon dioxide into formate in an aqueous system. The prepared electrodes are measured by Faradaic efficiency and partial current density for formate production. Electrocatalytic reduction experiments are carried out at -1.8 V (vs. Ag/AgCl) using H-type cell under ambient temperature and pressure and the gas and liquid products are analyzed by gas chromatograph and liquid chromatograph, respectively. As results, the Sn-Pb electrodes show higher Faradaic efficiency and partial current density than the single metal electrode. The Sn-Pb alloy electrode which have Sn:Pb molar ratio=2:1, shows the highest Faradaic efficiency of 88.7%.
목차
ABSTRACT
1. INTRODUCTION
2. EXPERIMENTAL
3. RESULTS AND DISCUSSIONS
4. CONCLUSION
REFERENCES
참고문헌 (11)
참고문헌 신청
[학술지(정기간행물)] - Alvarez-Guerra M. / 2014 / Continuous electrochemical reduction of carbon dioxide into formate using a tin cathode : Comparison with lead cathode / Chem Eng Res Des 92 : 692 ~ 701
[학위논문] - Choi SY. / 2015 / A study on the electrochemical reduction of carbon dioxide into formic acid using Sn-Pb alloy elec-trocatalysts / Chungnam National University
[학술지(정기간행물)] - Choi SY. / 2016 / Electrochemical reduction of carbon dioxide to formate on tin-lead alloys / ACS Sustainable Chem Eng 4 : 1311 ~ 1318
[학술지(정기간행물)] - Christophe J. / 2012 / Electro-reduction of carbon dioxide on copper-based electrodes : Activity of copper single crystals and copper-gold alloys / Electrocatal 3 : 139 ~ 146
[단행본] - Hori Y. / 2008 / Electrochemical CO 2 reduction on metal elec-trodes, in modern aspects of electrochemistry / Springer
[학위논문] - Choi SY. / 2015 / A study on the electrochemical reduction of carbon dioxide into formic acid using Sn-Pb alloy elec-trocatalysts / Chungnam National University
[학술지(정기간행물)] - Choi SY. / 2016 / Electrochemical reduction of carbon dioxide to formate on tin-lead alloys / ACS Sustainable Chem Eng 4 : 1311 ~ 1318
[학술지(정기간행물)] - Christophe J. / 2012 / Electro-reduction of carbon dioxide on copper-based electrodes : Activity of copper single crystals and copper-gold alloys / Electrocatal 3 : 139 ~ 146
[단행본] - Hori Y. / 2008 / Electrochemical CO 2 reduction on metal elec-trodes, in modern aspects of electrochemistry / Springer
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UCI(KEPA) : I410-ECN-0101-2017-453-001413490