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논문 기본 정보
- 자료유형
- 학술저널
- 저자정보
- 발행연도
- 2018.7
- 수록면
- 1 - 19 (19page)
- DOI
- 10.1186/s40580-018-0150-5
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초록· 키워드
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Manganese plays multiple role in many biological redox reactions in which it exists in different oxidation states from Mn(II) to Mn(IV). Among them the high-valent manganese-oxo intermediate plays important role in the activity of certain enzymes and lessons from the natural system provide inspiration for new developments of artificial systems for a sustainable energy supply and various organic conversions. This review describes recent advances and key lessons learned from the nature on high-valent Mn-oxo intermediates. Also we focus on the elemental science developed from the natural system, how the novel strategies are realised in nano particles and molecular sites at heterogeneous and homogeneous reaction conditions respectively. Finally, perspectives on the utilisation of the high-valent manganese-oxo species towards other organic reactions are proposed.
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참고문헌 (120)
참고문헌 신청
V. L. Pecoraro / 1994 / Interaction of manganese with dioxygen and its reduced derivatives / Chem. Rev 94:807~826
R. Manchanda / 1995 / High-valentoxomanganese clusters: structural and mechanistic work relevant to the oxygen-evolving center in photosystem II / Coord. Chem. Rev 144:1~38
G. C. Dismukes / 1996 / Manganese enzymes with binuclear active sites / Chem. Rev 96:2909~2926
C. F. Yocum / 1999 / Recent advances in the understanding of the biological chemistry of manganese / Curr. Opin. Chem. Biol 3:182~187
W. Zhu / 2017 / Biological functions controlled by manganese redox changes in mononuclear Mn-dependent enzyme / Essays Biochem 61:259~270
R. Manchanda / 1995 / High-valentoxomanganese clusters: structural and mechanistic work relevant to the oxygen-evolving center in photosystem II / Coord. Chem. Rev 144:1~38
G. C. Dismukes / 1996 / Manganese enzymes with binuclear active sites / Chem. Rev 96:2909~2926
C. F. Yocum / 1999 / Recent advances in the understanding of the biological chemistry of manganese / Curr. Opin. Chem. Biol 3:182~187
W. Zhu / 2017 / Biological functions controlled by manganese redox changes in mononuclear Mn-dependent enzyme / Essays Biochem 61:259~270
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