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초록· 키워드
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A theoretical model, based on the density functional theory, has been proposed to study the electrostatic adsorption of uniformly charged soft (penetrating inside each other) and hard spherical ions, where the charge is uniformly smeared on the surface and uniformly smeared inside a sphere. The proposed model explains the layering phenomenon arising from the packing effect of hard spherical ions regardless of the charge distribution of ions, and the results are comparable to Monte Carlo simulation data for the soft and hard spherical ions. The strong cross-correlation between the hard sphere contribution and Coulomb interaction appears at strongly surface-associated ion and depends on the size of ions, whereas the hard sphere contribution plays an important role in ionic adsorption at low charged ion. The charge distribution of ions strongly influence the local charge and particle densities; the sphere distribution, where the charge is uniformly smeared on the surface, shows higher particle density than the shell distribution, where the charge is uniformly smeared inside a sphere.
목차
I. INTRODUCTION
II. THEORETICAL BACKGROUND
III. RESULTS AND DISCUSSION
IV. CONCLUDING REMARKS
REFERENCES
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